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디아조크로마논과 보론산의 팔라듐 촉매하 결합반응을 이용한 Lespedezol A1의 합성

Formal Synthesis of Lespedezol A1 via Versatile Palladium-Catalyzed Cross-Coupling of Diazochromanone with Arylboronic Acid

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A formal synthesis of Lespedezol A1 has been accomplished. The key feature of this synthesis involves an effi- cient and powerful palladium-catalyzed cross coupling reaction of diazocarbonyl compound with bis(benzyloxy)phenylboronic acid for the key 3-aryl-chromen-4-one intermediate, which was difficult to be prepared by Suzuki coupling reaction in the previous study. The versatile and efficient synthetic procedure would facilitate synthesis of pterocarpenes and their deriv- atives.

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